1) Dr. Zhivago.
The music is as big as the story. I think this score stuck in people's minds in a way that converged the art of the film with the music in a bigger than life manner. The musical master Maurice Jarre wrote the score and was influenced under the direction of David Lean, who made many movies with him. Is Paris Burning, Ryan's Daughter and Lawrence of Arabia follow very close.
2) The Third Man.
Carol Reed's use of Anton Karas' zither music still haunts us when we think of movies walking down dark city streets.
3) A Hard Day's Night.
This still defines for many the use of pop music in film. In addition, in their other movie, Help, Richard Lester cleverly mixes in classical pieces.
Ron Grainer's score for to Sir With Love follows for me.
4) Mary Poppins.
Hands down the Sherman brothers win the gold. This is the perfect baby sitting movie for kids. Also, I think this was shot at the same studio and same time as A Hard Day's Night.
A few extra notes:
My favorite British composer is John Barry and his score for The Ipcress File would follow the Lean films.
While my favourite movie is Chariots of Fire and is emotively number one, I don't think it quite wove into the movie with the impact that Zhivago did. The story was bigger than the music. Nevertheless, Vangelis did an excellent job.
And, my definition of "all inclusive" for British film includes: location, characters, actors and directors and production company. While "Dr. Zhivago" was shot on the continent, I consider it British because of Lean and most of the cast, even though the story isn't and the money was put up by Carlo Ponti and MGM. Similar reason for "The Third Man." For "Mary Poppins" - British actors and shot in UK, eventhough it is a Disney film.

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