The second one down doesn't appear to be on a Bus route, could be Wigmore Street which as I recall has a slight gradient, looking towards the trees of Portman Square, or the other way round towards Cavendish Square.
Four locations from this episode still to find:
1: An art gallery/museum, and this is all you see of it.
2: London street
3: Quiet street where coffee is available outdoors
4: Street with antiques stalls
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The second one down doesn't appear to be on a Bus route, could be Wigmore Street which as I recall has a slight gradient, looking towards the trees of Portman Square, or the other way round towards Cavendish Square.